Metamagnetic phase transition in Mn5Si3 compound

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Abstract

The electrical resistance of the Mn5Si3 compound in magnetic fields up to 2 T at cryogenic temperatures in the range from 35 K to 90 K was studied. The characteristic temperatures of the magnetic phase transition TN1 and TN2 were determined based on the results of measuring the heat capacity at constant pressure CP, magnetization M and specific electrical resistance ρ. It was shown that the behavior of the ρ(T) curves differs depending on the measurement conditions and protocol. Based on the results of measuring the magnetocaloric properties in strong magnetic fields up to 10 T at cryogenic temperatures in the range from 25 to 125 K, both the inverse and conventional magnetocaloric effects were observed. The maximum value of the inverse magnetocaloric effect was ∆Tad = –1.1 K at an initial temperature T0 = 50 K in a magnetic field of 10 T. Conventional magnetocaloric effect with a maximum value of ∆Tad = +0.9 K is observed at T0 = 62.5 K in a field of 10 T. A local exponent of field distribution of entropy n is determined, the value of which n > 2 confirms the type and existence of a first-order phase transition.

About the authors

А. S. Kuznetsov

Kotelnikov Institute of Radio Engineering and Electronics of the RAS

Author for correspondence.
Email: kuznetsovalserg@gmail.com
Russian Federation, Mokhovaya St., 11, build. 7, Moscow, 125009

А. V. Mashirov

Kotelnikov Institute of Radio Engineering and Electronics of the RAS

Email: kuznetsovalserg@gmail.com
Russian Federation, Mokhovaya St., 11, build. 7, Moscow, 125009

I. I. Musabirov

Institute for Metals Superplasticity Problems of the RAS

Email: kuznetsovalserg@gmail.com
Russian Federation, Stepan Khalturin st., 39, Ufa, 450001

V. I. Mitsiuk

Scientific and Practical Center of the NAS of Belarus for Materials Science

Email: kuznetsovalserg@gmail.com
Belarus, Petrusya Brovka St., 19, build. 5, Minsk, 220072

А. V. Koshelev

Institute of Experimental Mineralogy of the RAS

Email: kuznetsovalserg@gmail.com
Russian Federation, Academician Osipyana St., 4, Chernogolovka, Moscow Region, 142432

К. А. Kolesov

Kotelnikov Institute of Radio Engineering and Electronics of the RAS

Email: kuznetsovalserg@gmail.com
Russian Federation, Mokhovaya St., 11, build. 7, Moscow, 125009

R. Yu. Gaifullin

Institute of Experimental Mineralogy of the RAS

Email: kuznetsovalserg@gmail.com
Russian Federation, Academician Osipyana St., 4, Chernogolovka, Moscow Region, 142432

V. V. Koledov

Kotelnikov Institute of Radio Engineering and Electronics of the RAS

Email: kuznetsovalserg@gmail.com
Russian Federation, Mokhovaya St., 11, build. 7, Moscow, 125009

V. G. Shavrov

Kotelnikov Institute of Radio Engineering and Electronics of the RAS

Email: kuznetsovalserg@gmail.com
Russian Federation, Mokhovaya St., 11, build. 7, Moscow, 125009

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